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Overcoming the Low-Surface-Energy-Induced Wettability Problem of Flexible and Transparent Electrodes for Large-Area Organic Photovoltaic Modules over 500 cm2

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Author(s)
Kwon Hyeok-Chan; Jeong Won; Lee Yang-Soo; Jang Jun-Ho; Jeong Hyeon-Seok; Kim Seungchan; Song Daehoon; Park Aeri; Noh Eunjee; Lee, Kwang Hee; Kang Hongkyu
Type
Article
Citation
Advanced Energy Materials, v.12, no.21
Issued Date
2022-06
Abstract
To realize the commercialization of nonfullerene acceptor-based efficient organic solar cells, a low-cost and indium-tin-oxide-free (ITO-free) flexible electrode-based module that can be produced by roll-to-roll production should be developed. However, the low surface energy of ITO-free electrodes hinders the formation of a uniform charge transport layer through solution processing; this is the main cause of the efficiency drop. Herein, the realization of a highly uniform ZnO bilayer on an ultrathin Ag film-based transparent electrode that is suitable for flexible substrates and large-area organic photovoltaic (OPV) module fabrication is demonstrated. Based on the sputtered ZnO and blade-coated ZnO nanoparticle-based electron transport bilayer, large OPV module areas of 528.5 and 108 cm(2) with high efficiencies of 7.67% and 9.15%, respectively, are achieved.
Publisher
Wiley-VCH Verlag
ISSN
1614-6832
DOI
10.1002/aenm.202200023
URI
https://scholar.gist.ac.kr/handle/local/10759
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