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Observation of mirror-odd and mirror-even spin texture in ultrathin epitaxially strained RuO2 films

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Author(s)
Zhang, Yichen; Jeong, Seung Gyo; Buiarelli, Luca; Lee, Seungjun; Guo, Yucheng; Wen, Jiaqin; Li, Hang; Nair, Sreejith; Choi, In Hyeok; Ren, Zheng; Yue, Ziqin; Hyun, Jounghoon; Zhang, Tieqiong; Fedorov, Alexei; Mo, Sung-Kwan; Lim, Hojoon; Hunt, Adrian; Waluyo, Iradwikanari; Kono, Junichiro; Minar, Jan; Lee, Jong Seok; Low, Tony; Birol, Turan; Fernandes, Rafael M.; Radovic, Milan; Jalan, Bharat; Yi, Ming
Type
Article
Citation
Science Advances, v.12, no.31
Issued Date
2026-07
Abstract
Recently, rutile ruthenium dioxide (RuO2) has attracted renewed interest due to expectations of prominent altermagnetic spin splitting. However, accumulating experimental evidence suggests that, in its bulk and thick-film forms, RuO2 does not display any form of magnetic ordering. Despite this, the spin structure of RuO2 remains largely unexplored in the ultrathin limit, where substrate-imposed epitaxial strain can be substantial. Here, we use spin-resolved angle-resolved photoemission spectroscopy, supported by ab initio calculations, to reveal the electronic structure of 2-nanometer-thick epitaxial RuO2 heterostructures. We observe an unconventional spin texture characterized by the coexistence of mirror-even and mirror-odd momentum-dependent components. A comprehensive symmetry analysis rules out nonmagnetic origins of this spin texture. These findings suggest an emergent nonrelativistic spin structure enabled by epitaxial strain in the ultrathin limit, marking a distinct departure from the behavior of relaxed or bulk RuO2. Our work opens previously unexplored perspectives for exploring symmetry-breaking mechanisms and spin textures in oxide heterostructures.
Publisher
American Association for the Advancement of Science
ISSN
2375-2548
DOI
10.1126/sciadv.aec2917
URI
https://scholar.gist.ac.kr/handle/local/34359
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