OAK

Metastable photo-induced superconductivity far above Tc

Metadata Downloads
Author(s)
Chattopadhyay, Sambuddha; Eckhardt, Christian J.; Kennes, Dante M.; Sentef, Michael A.; Shin, Dongbin; Rubio, Angel; Cavalleri, Andrea; Demler, Eugene A.; Michael, Marios H.
Type
Article
Citation
npj Quantum Materials, v.10, no.1
Issued Date
2025-03
Abstract
Inspired by the striking discovery of metastable superconductivity in K3C60 at 100K, far above Tc = 20 K, we discuss possible mechanisms for long-lived, photo-induced superconductivity. Starting from a model of optically-driven Raman phonons coupled to inter-band electronic transitions, we develop a microscopic mechanism for photo-controlling the pairing interaction. Leveraging this mechanism, we first investigate long-lived superconductivity arising from the thermodynamic metastable trapping of the driven phonon. We then propose an alternative route, where the superconducting gap created by an optical drive leads to a dynamical bottleneck in the equilibration of quasi-particles. We conclude by discussing the implications of both scenarios for experiments that can be used to discriminate between them. Our work provides falsifiable explanations for the nanosecond-scale photo-induced superconductivity found in K3C60, while simultaneously offering a theoretical basis for exploring metastable superconductivity in other quantum materials. © The Author(s) 2025.
Publisher
Nature Research
ISSN
2397-4648
DOI
10.1038/s41535-025-00750-x
URI
https://scholar.gist.ac.kr/handle/local/18735
공개 및 라이선스
  • 공개 구분공개
파일 목록
  • 관련 파일이 존재하지 않습니다.

Items in Repository are protected by copyright, with all rights reserved, unless otherwise indicated.