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Enhanced infrared magneto-optical response of the nonmagnetic semiconductor BiTeI driven by bulk rashba splitting

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Author(s)
Demkó, L.; Schober, G.A.H.; Kocsis, V.; Bahramy, M.S.; Murakawa, H.; Lee, Jong Seok; Kézsmárki, I.; Arita, R.; Nagaosa, N.; Tokura, Y.
Type
Article
Citation
Physical Review Letters, v.109, no.16
Issued Date
2012-12
Abstract
We study the magneto-optical (MO) response of the polar semiconductor BiTeI with giant bulk Rashba spin splitting at various carrier densities. Despite being nonmagnetic, the material is found to yield a huge MO activity in the infrared region under moderate magnetic fields (up to 3T). Our first-principles calculations show that the enhanced MO response of BiTeI comes mainly from the intraband transitions between the Rashba-split bulk conduction bands. These transitions connecting electronic states with opposite spin directions become active due to the presence of strong spin-orbit interaction and give rise to distinct features in the MO spectra with a systematic doping dependence. We predict an even more pronounced enhancement in the low-energy MO response and dc Hall effect near the crossing (Dirac) point of the conduction bands. © 2012 American Physical Society.
Publisher
American Physical Society
ISSN
0031-9007
DOI
10.1103/PhysRevLett.109.167401
URI
https://scholar.gist.ac.kr/handle/local/15735
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