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Slot die coated planar perovskite solar cells via blowing and heating assisted one step deposition

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Author(s)
Kim, Jueng-Eun; Jung, Yen-Sook; Heo, Youn-Jung; Hwang, Kyeongil; Qin, Tianshi; Kim, Dong-Yu; Vak, Doojin
Type
Article
Citation
Solar Energy Materials and Solar Cells, v.179, pp.80 - 86
Issued Date
2018-06
Abstract
CH3NH3PbI3-based planar perovskite solar cells were fabricated by slot-die coating, a scalable method. Slot-die coating tends to produce perovskite layers with much lower coverage with overgrown crystals than spin coating, which does not include a self-drying mechanism in the process. To mimic the self-drying behavior inherent in spin coating, the present study introduces a blowing step in the slot-die coating method, which significiltly improved coverage of the prepared slot-die coated perovskite films. The slot-die-coated device with blowing showed a moderate power conversion efficiency (PCE) of 8.8%. The morphology of the slot-die-coated perovskite film is further improved by optimizing the deposition temperature. The combination of blowing rand heating during the slot-die-coating step and the introduction of a printing-friendly hole transport layer resulted in a PCE of 12.7% for the devices fabricated in air.
Publisher
Elsevier BV
ISSN
0927-0248
DOI
10.1016/j.solmat.2018.02.003
URI
https://scholar.gist.ac.kr/handle/local/13254
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