Large anomalous Hall effect and intrinsic Berry curvature in magnetic Weyl semimetal NdAlGe

Abstract

Weyl semimetals driven by both time-reversal (TRS) and inversion symmetries (IS) are rare and be a good platform to investigate the relationship between chiral current and magnetic order. NdAlGe compound, grown in a single crystalline form by the flux method, has a noncentrosymmetric I41md crystal structure, which breaks inversion symmetry. The magnetic susceptibility χ(T) shows anisotropic behavior; ferromagnetic with divergence of field cooling (FC) and zero field cooling (ZFC) in H∥c, and antiferromagnetic transition for magnetic field H⊥c. The band structure calculation has revealed that NdAlGe is the type-II Weyl semimetal with four types of Weyl nodes in the ab-plane with a probable Fermi surface nesting vector. The ferromagnetic spin alignment gives a significant anomalous Hall coefficient Rs and large anomalous Hall conductivity σxy A, for H∥c. The giant anomalous Hall conductivity σxy A, constant SH=σxy A/M (H = 50 kOe) value, and their Karplus and Luttinger (KL) analysis support that the giant AHE is associated with the intrinsic Berry curvature in NdAlGe compound. The intrinsic Berry curvature is also confirmed by the planar Hall effect over a wide temperature range, implying that the Weyl semimetallic property is not relevant with the magnetic order. © 2023 Elsevier Ltd